Journal of the Physical Society of Japan
Online ISSN : 1347-4073
Print ISSN : 0031-9015
ISSN-L : 0031-9015
Evidence for Magnetic-Field-Induced Quadrupolar Ordering in the Heavy-Fermion Superconductor PrOs4Sb12
Masahumi KohgiKazuaki IwasaMotoki NakajimaNaoto MetokiShingo ArakiNick BernhoeftJean-Michel MignotArsen GukasovHideyuki SatoYuji AokiHitoshi Sugawara
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2003 Volume 72 Issue 5 Pages 1002-1005

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Abstract

Neutron diffraction experiments on the heavy-fermion superconductor PrOs4Sb12 revealed that a small antiferromagnetic moment, parallel to [010] (y-direction), is induced in the field-induced phase (H||z). The analysis, based on the Γ1 singlet ground state crystal field model, shows that antiferro-order of Oyz-type quadrupole moments of Pr ions is formed in the field-induced phase. This strongly suggests that the crystal field ground-state of Pr ions in PrOs4Sb12 is the Γ1 singlet and the quadrupolar ordering is induced due to level crossing with an excited state under a magnetic field.

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© The Physical Society of Japan 2003
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